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Jenny, there are a number of buses a day from Santo Domingo to Burgos - and then from there to Leon on ALSA.
Santo Domingo is on the Logroño to Burgos line on Jiminez http://www.autobusesjimenez.com/ - You can only book tickets on this both one month in advance (not earlier).
There is one bus per day on ALSA from Santo Domingo to Leon
05:10 08:45 SANTO DOMINGO DE LA CALZADA LEON 3h 35m 15,69 €
Do you know if this bus is still running as i need to get from Santo Domingo to Leon in April will they take Bicycles?